Season One

Jill St. John as Molly.
Episodes; "Hi Diddle Riddle/Smack In The Middle".
Villain : The Riddler
She became the only person to die in the batcave, also she was of course the first moll ever. Don't forget, without her the batusi wouldn't have been possible!
Picture above from : http://catwomanfan.com/en/other_ladies/jsj/index.php (highly recommend this site, loads of information and pictures for Jill St. John)

Nancy Kovack as Queenie.
Episodes; "The Joker's Wild/Batman's Riled"
Villain : The Joker

Susan Silo as Mousey
Episodes; "A Ridller A Day Keeps The Riddler Away/When The Rat's Away The Mice Will Play"
Villain : The Riddler

Diane McBain as Lisa.
Episodes : "The Thirteenth Hat/Batman Stand's Pat"
Villain : The Mad Hatter

Donna Loren as Susie
Episodes : "The Joker Goes To School/He Meets His Match The Grisly Ghoul"
Villain : The Joker
Susie is a cheerleader at Dick Grayson's school, she later see's her wrong doing's after the Joker attempts to murder her with poisoned perfume but Batman save's her. She's the first example of a re-hibilitated moll.

Myrna Fahey as Blaze
Episodes : "True Or False Face/Holy Rat Race"
Villain : False Face

Linda Gaye Scott as Moth
Episodes : "A Ring Of Wax/Give 'Em The Axe"
Villain : The Riddler
See's that "crime dosent pay" at the end of the second part, but Batman tells her she's too late.

Jane Wald as Jill
Episodes : "The Joker Trumps An Ace/Batman Sets The Pace"
Villain : The Joker

Ziva Rodann as Queen Nefertiti
Episodes : "The Curse Of Tut/The Pharoah's In A Rut"
Villain : King Tut

Francine York as Lydia Limpet
Episodes "The Bookworm Turns/As Gotham City Burn's"
Villain : The Bookworm

Sherry Jackson as Pauline
Episodes : "Death In Slow Motion/The Riddler's False Notion"
Villain : The Riddler

Julie Gregg as Finella
Episodes : "Fine Finny Fiends/Batman Makes The Scenes"
Villain : The Penguin